Carbonate Esters and Additives Analysis in Li-ion Battery

This application note presents a reliable, user-friendly, and cost-effective solution to meet the demand for carbonate esters and additives analysis. The solution was developed using the Agilent 8860/8890 GC system with a split-splitless injector and a flame ionization detector (FID).

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Analysis of Carbonate Esters and Additives in Battery Electrolyte Using Agilent 8860/8890

The demand for electric vehicles and energy storage systems worldwide has been growing significantly and is expected to expand rapidly.

The organic solution inside the battery, known as an electrolyte, acts as an ion carrier and facilitates the movement of ions from the cathode to the anode. Liquid electrolytes' capacity, cycle, life, and stability are greatly influenced by the composition, proportion, and purity of their solvent and additives. These solvents are expected to decompose at low potentials, resulting in lower cell performance. To monitor the performance, we need to analyze different chemical compositions in the cell.
The Agilent 8860/8890 equipped with FID will give the composition of different species present in the Lithium-ion Batteries.
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GBA Analyzer features

  • Fast compositional analysis of different Carbonate Esters
  • Excellent Repeatability & Reproducibility
  • Total runtime under 15 mins
  • Full hardware and software turnkey solution
  • Automatic Liquid Sampler (ALS) for precise sample injection
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Results and discussion

Target compounds behavior in GC chromatogram

To observe the behavior of the target compounds on the GC chromatogram, a standard mixture with a concentration of 200 mg/L was analyzed using both helium and nitrogen as the carrier gas (see Figure 1). All compounds could elute from the GC column within 14 minutes and achieved baseline separation. It was observed that the retention times of all compounds were earlier with nitrogen as the carrier gas (Figure 1B) compared to helium (Figure 1A).

Calibration curve and linearity

The responses of each compound were evaluated at six concentration levels using the calibration standards prepared in this study. The results obtained using helium as the carrier gas were collected and statistically analyzed. The calibration curves for the 13 compounds are shown in Figure 2. All 13 compounds exhibited strong positive linear correlations between peak area and concentration, with correlation coefficients (R2) ranging from 0.9996 to 0.9999.

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